Doctor of Philosophy, The Ohio State University, 2019, Environmental Science
Reducing carbon dioxide (CO2) emissions is one of the most pressing issues facing the electricity system. Towards this end, prior work investigated generating electricity with geologically stored CO2 by using it to extract heat from sedimentary basins geothermal resources. This dissertation expands on this idea by developing and valuing approaches for CO2-based energy storage.
In the first chapter, we investigate the value that three bulk energy storage (BES) approaches have for reducing system-wide CO2 emissions and water requirements: CO2-Bulk Energy Storage (CO2-BES), which is a CO2-based energy storage approach that uses a concentric-ring, pressure based (CRP-BES) design, Pumped Hydro Energy Storage (PHES), and Compressed Air Energy Storage (CAES). Our results suggest that BES could decrease system-wide CO2 emissions by increasing the utilization of wind, but it can also alter the dispatch order of regional electricity systems in other ways (e.g., increase in the utilization of natural gas power capacity and of coal power capacity, decrease in the utilization of nuclear power capacity). While some changes provide negative value (e.g., decrease in nuclear increased CO2 emission), the system-wide values can be greater than operating cost of BES.
In the second and third chapters, we investigate two mechanisms for using CO2 for energy storage: storage of (1) pressure and (2) heat. For pressure storage, we investigated the efficacy of the CO2-BES system using the CRP-BES design over cycles of varying durations. We found that CO2-BES could time-shift up to a couple weeks of electricity, but the system cannot frequently dispatch electricity for longer durations than was stored. Also, the cycle duration does not substantially affect the power storage capacity and power output capacity if the total time spent charging, discharging, or idling is equal over a multi-year period. For thermal energy storage, we investigated the efficacy of using pre-heated CO2 and pre-h (open full item for complete abstract)
Committee: Jeffrey Bielicki (Advisor); Ramteen Sioshansi (Committee Member); Gil Bohrer (Committee Member); Brent Sohngen (Committee Member)
Subjects: Alternative Energy; Energy; Engineering; Environmental Economics; Environmental Science