Skip to Main Content
 

Global Search Box

 
 
 
 

ETD Abstract Container

Abstract Header

Synthesis of Benzoxazoles Containing Allyl Crosslinking Sites via Claisen Rearrangements

Hutson, Leslie K.

Abstract Details

1999, Master of Science (MS), Wright State University, Chemistry.
Hutson, Leslie K. M.S. Department of Chemistry, Wright State University, 1999. Synthesis of Benzoxazoles Containing Allyl Crosslinking Sites via Claisen Rearrangements. The reaction of diethyl 2,5-dihydroxyterephthalate with allyl bromide/K2CO3 in DMF followed by hydrolysis provided 2,5-di(allyloxy)terephthalic acid. The conversion of 2,5-di (allyloxy)terephthalic acid to 1,4-di(2-benzoxazolyl)-2,5-di(allyloxy)benzene in PPSE was unsuccessful. However, the reaction of 1,4-di(2-benzoxazolyl)-2,5- dihydroxybenzene with allyl bromide/K2CO3 provided 1,4-di(2-benzoxazolyl)-2,5- di(allyloxy)benzene. DSC analysis indicated that 1,4-di(2-benzoxazolyl)-2,5- di(allyloxy)benzene undergoes a Claisen rearrangement to the corresponding diallyl product. The synthesis of 2-allyloxy-1,4-di(2-benzoxazolyl)benzene was carried out using 2-hydroxy-1,4-di(2-benzoxazolyl)benzene as starting material. DSC analysis was inconclusive with respect to a Claisen rearrangement. The reaction of 2-allyloxybenzoic acid with 2,2-bis(3-amino-4-hydroxyphenyl)-1,1,1,3,3,3-hexafluoropropane in PPSE was unsuccessful but the reaction of 2,2-bis(2-(2-hydroxyphenyl)-5-benzoxazolyl)-1,1,1,3,3,3-hexafluoropropane with allyl bromide/K2CO3 in DMF provided 2,2-bis(2-(2- allyloxyphenyl)-5-benzoxazolyl)-1,1,1,3,3,3-hexafluoropropane. DSC analysis of 2,2- bis(2-(2-allyloxyphenyl)-5-benzoxazolyl)-1,1,1,3,3,3-hexafluoropropane was inconclusive as to the presence of a Claisen rearrangement.
William Feld (Advisor)
57 p.

Recommended Citations

Citations

  • Hutson, L. K. (1999). Synthesis of Benzoxazoles Containing Allyl Crosslinking Sites via Claisen Rearrangements [Master's thesis, Wright State University]. OhioLINK Electronic Theses and Dissertations Center. http://rave.ohiolink.edu/etdc/view?acc_num=wright974400715

    APA Style (7th edition)

  • Hutson, Leslie. Synthesis of Benzoxazoles Containing Allyl Crosslinking Sites via Claisen Rearrangements. 1999. Wright State University, Master's thesis. OhioLINK Electronic Theses and Dissertations Center, http://rave.ohiolink.edu/etdc/view?acc_num=wright974400715.

    MLA Style (8th edition)

  • Hutson, Leslie. "Synthesis of Benzoxazoles Containing Allyl Crosslinking Sites via Claisen Rearrangements." Master's thesis, Wright State University, 1999. http://rave.ohiolink.edu/etdc/view?acc_num=wright974400715

    Chicago Manual of Style (17th edition)